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Self-healing hypercrosslinked metal–organic polyhedra (HCMOPs) membranes with antimicrobial activity and highly selective separation properties

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dc.contributor.author Liu, Jinjin
dc.contributor.author Duan, Wenjie
dc.contributor.author Song, Jie
dc.contributor.author Guo, Xiuxiu
dc.contributor.author Wang, Zhifang
dc.contributor.author Shi, Xinlei
dc.contributor.author Liang, Jiajie
dc.contributor.author Wang, Juan
dc.contributor.author Cheng, Peng
dc.contributor.author Zaworotko, Michael J.
dc.contributor.author Zhang, Zhenjie
dc.date.accessioned 2019-10-07T10:58:24Z
dc.date.issued 2019
dc.identifier.uri http://hdl.handle.net/10344/8110
dc.description peer-reviewed en_US
dc.description.abstract Fabrication of hybrid membranes composed of porous materials embedded in polymer matrices is a subject of topical interest. Herein, we introduce a new class of hybrid membranes: hypercrosslinked metal-organic polyhedra (HCMOPs). These membranes are based upon soluble MOPs that can serve as high-connectivity nodes in hypercrosslinked polymer networks. HCMOPs spontaneously form macro-scale, defect-free, freestanding membranes and, thanks to the covalent cross-linking of MOPs, the resulting membranes possess multiple functionalities: strong water permeability; self-healing ability; antimicrobial activity; better separation and mechanical performance than pristine polyimine membranes. This study introduces a new concept for the design and fabrication of multi-functional membranes and also broadens the applications of MOPs en_US
dc.language.iso eng en_US
dc.publisher American Chemical Society en_US
dc.relation 16IA4624 en_US
dc.relation.ispartofseries Journal of the American Chemical Society;141 (30), pp. 12064-
dc.relation.uri https://dx.doi.org/10.1021/jacs.9b05155
dc.rights © 2019 ACS This document is the Accepted Manuscript version of a Published Work that appeared in final form in Journal of the American Chemical Society , copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://dx.doi.org/10.1021/jacs.9b05155 en_US
dc.subject hybrid membranes en_US
dc.subject HCMOPs en_US
dc.title Self-healing hypercrosslinked metal–organic polyhedra (HCMOPs) membranes with antimicrobial activity and highly selective separation properties en_US
dc.type info:eu-repo/semantics/article en_US
dc.type.supercollection all_ul_research en_US
dc.type.supercollection ul_published_reviewed en_US
dc.identifier.doi 10.1021/jacs.9b05155
dc.contributor.sponsor National Key Research and Development Program of China en_US
dc.contributor.sponsor National Natural Science Foundation of China en_US
dc.contributor.sponsor SFI en_US
dc.relation.projectid 2018YFA001800 en_US
dc.relation.projectid 21601093 en_US
dc.relation.projectid 16/IA/4624 en_US
dc.date.embargoEndDate 2020-07-09
dc.embargo.terms 2020-07-09 en_US
dc.rights.accessrights info:eu-repo/semantics/openAccess en_US


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